J Am Chem Soc August 2022 PMID 35862699

Cooperative Catalysis of Vibrationally Excited CO and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation.

Dae-Yeong Kim, Hyungwon Ham, Xiaozhong Chen, Shuai Liu, Haoran Xu, Bang Lu, Shinya Furukawa, Hyun-Ha Kim, Satoru Takakusagi, Koichi Sasaki, Tomohiro Nozaki

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Mentions

34
Peak: 16 in Jul 2022
across 4 sources since Jul 2022

Extended reach

658,025
potential audience

Total likes

45

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4,097

Mentions per month

Jul 2022 – Aug 2022

Where it's discussed

  • X / Twitter15 posts
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  • YouTube2 videos
  • Blogs2 articles

AI synopsis

What people are saying

The discussions convey high interest and recognition of the research's significance, with terms like 'breaks the thermodynamic limit' and 'catalysis breakthrough' illustrating excitement and importance. Participants reference specific techniques, such as plasma assistance and alloy catalysts, indicating deep engagement with the scientific content, which underscores the perceived high impact of the publication.

AgreementModerate agreement

Most discussions recognize the significance of the research, with many emphasizing its potential to break conventional limitations, though some remain cautious or neutral.

InterestHigh interest

The discussions reflect high interest, highlighted by enthusiastic words like 'breaks the limitation' and 'significant advances,' showing engagement with the breakthrough nature of the findings.

EngagementModerate engagement

Participants reference specific scientific concepts, such as plasma-assisted catalysis and vibrational excitation, indicating active engagement and familiarity with the research details.

ImpactHigh impact

The social discussions suggest the research could have substantial influence on catalysis and energy conversion fields, labeling it as 'game-changing' and emphasizing its potential to advance electrified chemical processes.

Abstract in brief

  • This study explores how nonthermal plasma (NTP) can significantly boost CO hydrogenation on PdGaSiO alloy catalysts, breaking the usual thermodynamic limits and achieving over twice the conversion rate compared to thermal processes.
  • Through advanced spectroscopy and structural analysis, the research shows that NTP activates vibrationally excited CO and prevents catalyst restructuring, with these excited CO molecules directly reacting with hydrogen on Pd sites to form valuable chemicals.
  • Combining experimental results with density functional theory (DFT) calculations, the work reveals that plasma-activated hydrogen accelerates formate formation and decomposition, offering new pathways for designing catalysts for electrified chemical processes.]

Top posts

Most liked on X and Bluesky
Top Science
@isciverse · X

Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_C_S @isciverse #Chemistry #ChemTwitter #scicomm #news #Technology #Tech #NewsBreak #Trending #research #AcademicTwitter #science https://t.co/MvL7lsCu2o https://t.co/qlb1Iui6BH

Jul 22, 2022 · 12 likes · 5 shares · 40,412 followers View post →
Phys.org Chemistry
@physorg_chem · X

Nonthermal plasma-promoted CO2 #hydrogenation in presence of alloy catalysts @HokkaidoUni @J_A_C_S https://t.co/L3hMYFrHcl https://t.co/9jfV66srOw

Jul 22, 2022 · 9 likes · 1 share · 7,197 followers View post →
JST CREST・さきがけ・ACT-X
@JST_Kisokenkyu · X

“Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation” by Kim Daeyeong, Ham Hyungwon, Chen Xiaozhong, et al., out in @J_A_C_S https://t.co/Qt5G6BeDzW

Jul 25, 2022 · 3 likes · 2 shares · 13,019 followers View post →
J. Am. Chem. Soc.
@J_A_C_S · X

Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation @HokkaidoUni @tokyotech_en #Cooperative #Catalysis #VibrationallyExcited #CO2 #Alloy #Thermodynamic #Limitation https://t.co/EypGExRmbh

Jul 22, 2022 · 2 likes · 185,565 followers View post →
Institute for Catalysis (ICAT) / 北海道大学触媒科学研究所
@ICAT_Hokudai · X

【Press Release】”Plasma-assisted catalysis for highly efficient CO2 utilization”(Associate Professor Shinya Furukawa, Catalyst Material Research Div.,Associate Professor Satoru Takakusagi, Catalyst Surface Research Div.) https://t.co/mZ3npbWAgJ https://t.co/jUkZs6pjr1

Aug 23, 2022 · 2 likes · 329 followers View post →
JST CREST・さきがけ・ACT-X
@JST_Kisokenkyu · X

CREST「革新的反応」領域、野崎智洋先生らの成果です。 プラズマを作用させることでCO2還元反応効率を向上させるとともに、その反応系の触媒とプラズマの協奏効果の観測にも成功し、Journal of the American Chemical Societyに報告しています。 https://t.co/Qt5G6BeDzW

Jul 25, 2022 · 1 like · 1 share · 13,019 followers View post →

All mentions

Institute for Catalysis (ICAT) / 北海道大学触媒科学研究所
@ICAT_Hokudai · X

【Press Release】”Plasma-assisted catalysis for highly efficient CO2 utilization”(Associate Professor Shinya Furukawa, Catalyst Material Research Div.,Associate Professor Satoru Takakusagi, Catalyst Surface Research Div.) https://t.co/mZ3npbWAgJ https://t.co/jUkZs6pjr1

Aug 23, 2022 · 2 likes · 329 followers View post →
しじみ
@Shijimijp · X

RT @JST_Kisokenkyu: CREST「革新的反応」領域、野崎智洋先生らの成果です。 プラズマを作用させることでCO2還元反応効率を向上させるとともに、その反応系の触媒とプラズマの協奏効果の観測にも成功し、Journal of the American Chemi…

Jul 26, 2022 · 1 share · 159 followers View post →
副鼻腔炎経過順調
@tet__yam · X

RT @JST_Kisokenkyu: “Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation”…

Jul 25, 2022 · 2 shares · 602 followers View post →
J. Am. Chem. Soc.
@J_A_C_S · X

RT @JST_Kisokenkyu: “Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation”…

Jul 25, 2022 · 2 shares · 185,565 followers View post →
JST CREST・さきがけ・ACT-X
@JST_Kisokenkyu · X

“Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation” by Kim Daeyeong, Ham Hyungwon, Chen Xiaozhong, et al., out in @J_A_C_S https://t.co/Qt5G6BeDzW

Jul 25, 2022 · 3 likes · 2 shares · 13,019 followers View post →
JST CREST・さきがけ・ACT-X
@JST_Kisokenkyu · X

CREST「革新的反応」領域、野崎智洋先生らの成果です。 プラズマを作用させることでCO2還元反応効率を向上させるとともに、その反応系の触媒とプラズマの協奏効果の観測にも成功し、Journal of the American Chemical Societyに報告しています。 https://t.co/Qt5G6BeDzW

Jul 25, 2022 · 1 like · 1 share · 13,019 followers View post →
ScienceStop
@B0tSci · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 24, 2022 · 5 shares · 4,074 followers View post →
J. Am. Chem. Soc.
@J_A_C_S · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 24, 2022 · 5 shares · 185,565 followers View post →
Phys.org Chemistry
@physorg_chem · X

Nonthermal plasma-promoted CO2 #hydrogenation in presence of alloy catalysts @HokkaidoUni @J_A_C_S https://t.co/L3hMYFrHcl https://t.co/9jfV66srOw

Jul 22, 2022 · 9 likes · 1 share · 7,197 followers View post →
xxy
@xxy07255392 · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 22, 2022 · 5 shares · 264 followers View post →
J. Am. Chem. Soc.
@J_A_C_S · X

Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation @HokkaidoUni @tokyotech_en #Cooperative #Catalysis #VibrationallyExcited #CO2 #Alloy #Thermodynamic #Limitation https://t.co/EypGExRmbh

Jul 22, 2022 · 2 likes · 185,565 followers View post →
Diversity News Magazine
@RealDNewsMag · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 22, 2022 · 5 shares · 10,904 followers View post →
Academic Chatter
@workingbnb · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 22, 2022 · 5 shares · 3,093 followers View post →
ScienceStop
@B0tSci · X

RT @isciverse: Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_…

Jul 22, 2022 · 5 shares · 4,074 followers View post →
Top Science
@isciverse · X

Cooperative Catalysis of Vibrationally Excited CO2 and Alloy Catalyst Breaks the Thermodynamic Equilibrium Limitation. @J_A_C_S @isciverse #Chemistry #ChemTwitter #scicomm #news #Technology #Tech #NewsBreak #Trending #research #AcademicTwitter #science https://t.co/MvL7lsCu2o https://t.co/qlb1Iui6BH

Jul 22, 2022 · 12 likes · 5 shares · 40,412 followers View post →