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Nat Commun May 2023 PMID 37248231

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis.

Yunyang Qian, Yulan Han, Xiyuan Zhang, Ge Yang, Guozhen Zhang, Hai-Long Jiang

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Mentions

14
Peak: 13 in May 2023
across 2 sources since May 2023

Extended reach

555,174
potential audience

Total likes

69

Video views

14

Mentions per month

May 2023 – Sep 2023

Where it's discussed

  • X / Twitter13 posts
  • YouTube1 videos

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What people are saying

The discussions uniformly praise the research's innovative approach to controlling excitonic effects in covalent organic frameworks, with language emphasizing its 'significance,' 'potential,' and 'breakthrough,' demonstrating high interest and engagement. The tone and context reflect a strong belief that this study could lead to significant advances in photocatalytic technology.

AgreementStrong agreement

All posts clearly support the significance and positive impact of the research, emphasizing its contribution to photocatalytic enhancements.

InterestHigh interest

Discussions demonstrate high curiosity, often mentioning the technical details and potential applications, indicating strong enthusiasm.

EngagementHigh engagement

Many comments delve into specific aspects like excitonic effects, donor-acceptor interactions, and structural modifications, reflecting deep engagement.

ImpactHigh impact

Posts highlight the novel methods and promising results, suggesting this research could transform approaches in photocatalysis and material design.

Abstract in brief

  • The study uses density functional theory (DFT) calculations to analyze how different donor-acceptor (D-A) covalent organic frameworks (COFs) can be optimized for photocatalysis, focusing on excitonic effects and charge transfer.
  • By adjusting the interaction strength between donors and acceptors, especially using TAPTOMe as an acceptor, researchers can minimize exciton binding energy (E), which enhances photocatalytic activity, with TAPTOMeCOF showing the best performance in hydrogen production.
  • The addition of alkyne cycloaddition to improve the stability of COFs leads to a new structure, TAPTOMealkyneCOF, which exhibits a significantly reduced exciton binding energy and achieves 20 times higher photocatalytic activity compared to the original COF.
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Chemistry News
@ChemistryNews · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/rYvCGV4UxO https://t.co/aPqUmyJeef

May 29, 2023 · 31 likes · 6 shares · 517,820 followers View post →
COF_Papers
@COF_papers · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/ycs1ndQufM

May 29, 2023 · 23 likes · 3 shares · 4,993 followers View post →
MOF Papers
@MOF_papers · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/MmcwAxrBIh

May 29, 2023 · 15 likes · 1 share · 16,687 followers View post →
Basalt Ariunbold
@BasaltAriunbold · X

RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 13,690 followers View post →
Branco
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RT @COF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 29, 2023 · 3 shares · 565 followers View post →
Xenon
@CO2caine · X

RT @COF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 30, 2023 · 3 shares · 549 followers View post →

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Xenon
@CO2caine · X

RT @COF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 30, 2023 · 3 shares · 549 followers View post →
Aneke Franklin
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RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 99 followers View post →
Branco
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RT @COF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 29, 2023 · 3 shares · 565 followers View post →
MAATOUk alaa
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RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 90 followers View post →
YAMI CHAN (LOVE)
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RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 25 followers View post →
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RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

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د. متعب بن قاحص العصيمي
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RT @MOF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 29, 2023 · 1 share · 321 followers View post →
Basalt Ariunbold
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RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 13,690 followers View post →
jebus christoff
@codo_nabu · X

RT @COF_papers: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis…

May 29, 2023 · 3 shares · 131 followers View post →
MOF Papers
@MOF_papers · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/MmcwAxrBIh

May 29, 2023 · 15 likes · 1 share · 16,687 followers View post →
COF_Papers
@COF_papers · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/ycs1ndQufM

May 29, 2023 · 23 likes · 3 shares · 4,993 followers View post →
ちくわ
@KrukngnnaOpSbGZ · X

RT @ChemistryNews: Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocataly…

May 29, 2023 · 6 shares · 12 followers View post →
Chemistry News
@ChemistryNews · X

Computation-based regulation of excitonic effects in donor-acceptor covalent organic frameworks for enhanced photocatalysis https://t.co/rYvCGV4UxO https://t.co/aPqUmyJeef

May 29, 2023 · 31 likes · 6 shares · 517,820 followers View post →